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CHEN Xiao-bo, LI Song, ZHAO Guo-ying, LIU Hong-Zhen, GUO Jing-hua, MA Yu, WANG Ke-zhi, GENG Zhu-feng. Luminescence enhancement mechanism of Er3+ ion by Ag@SiO2 core-shell nanostructure in Tellurite glass[J]. Chinese Optics. doi: 10.37188/CO.2021-0142
Citation: CHEN Xiao-bo, LI Song, ZHAO Guo-ying, LIU Hong-Zhen, GUO Jing-hua, MA Yu, WANG Ke-zhi, GENG Zhu-feng. Luminescence enhancement mechanism of Er3+ ion by Ag@SiO2 core-shell nanostructure in Tellurite glass[J]. Chinese Optics. doi: 10.37188/CO.2021-0142

Luminescence enhancement mechanism of Er3+ ion by Ag@SiO2 core-shell nanostructure in Tellurite glass

doi: 10.37188/CO.2021-0142
Funds:  Project supported by the National Natural Science Foundation of China (No. 51972020 and No. 51472028);
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  • Corresponding author: chen78xb@sina.com
  • Accepted Date: 2021-11-18
  • Available Online: 2021-11-18
  • In present manuscript, we introduce the prepared Ag@SiO2 nanostructure directly into tellurite luminescence glass 70TeO2-25ZnO-5La2O3-0.5Er2O3. We find that the maximum enhancement of visible and infrared excitation spectra intensity of (A) Ag(1.6×10−6 mol /L)@SiO2(40 nm) @Er3+(0.5%):tellurite glass relative to (B) Er3+(0.5%):tellurite glass is about 149.0% and 161.5% respectively. Their maximum enhancement of visible and infrared luminescence spectra intensity is 155.2% and 151.6%, respectively. We also find that sample (A) has a large increase for lifetime compared with sample (B). Because surface plasmon absorption peak of Ag@SiO2 is located just at 546.0 nm, it completely resonates with the luminescence peak of erbium ion at 546.0 nm. Therefore, the resonance enhancement action of Ag@SiO2 on the luminescence of erbium-doped tellurite luminescence glass is obvious. The Ag@SiO2 nano core-shell structure studied in present paper is pre-fabricated in advance. Thanks to advantages of the step-by-step realization of the silver nano core-shell structure and the production of glass: it can successfully smoothly control the size of Ag@SiO2, it also has the advantage of strong operability in the manufacturing process of Ag@SiO2@Er:telluride luminescence glass. It also has the advantages of low price and minor cost. Moreover, it can not only ensure that the silver is not oxidized, but also it can successfully control the distance between the rare earth ion luminescence center and the silver surface plasma, and it can also successfully reduce the back energy transfer, therefore which promotes the silver surface plasma to more effectively enhance the intensity of photo-luminescence. These results are of great significance for enhancing the luminescence intensity of rare earth luminescent materials and promoting their wider application prospects.
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